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Response of indigenous Cd-tolerant electrochemically active bacteria in MECs toward exotic Cr(VI) based

Xia Hou, Liping Huang, Peng Zhou, Hua Xue, Ning Li

《环境科学与工程前沿(英文)》 2018年 第12卷 第4期 doi: 10.1007/s11783-018-1057-4

摘要:

Cell membrane of indigenous Cd-tolerant EAB harbored more cadmium than chromium.

Indigenous Cd-tolerant EAB cytoplasm located more chromium than cadmium.

Simultaneously quantitatively imaging Cd(II) and Cr(III) ions in EAB was achieved.

Current accelerated the harboring of cadmium in EAB at an initial 2 h.

Current directed the accumulation of more chromium in EAB over time.

关键词: Microbial electrolysis cell     Electrochemically active bacteria     Cd-tolerant bacteria     Cd(II) and Cr(VI)     Fluorescence probe    

An antibiotic composite electrode for improving the sensitivity of electrochemically active biofilm biosensor

《环境科学与工程前沿(英文)》 2022年 第16卷 第8期 doi: 10.1007/s11783-022-1518-7

摘要:

• Antibiotic azithromycin employed in graphite electrode for EAB biosensor.

关键词: AZM@GP composite electrode     EAB-biosensor     Water quality early-warning    

Optimization of electrochemically synthesized Cu

Kasra Pirzadeh, Ali Asghar Ghoreyshi, Mostafa Rahimnejad, Maedeh Mohammadi

《化学科学与工程前沿(英文)》 2020年 第14卷 第2期   页码 233-247 doi: 10.1007/s11705-019-1893-1

摘要: Cu (BTC) , a common type of metal organic framework (MOF), was synthesized through electrochemical route for CO capture and its separation from N . Taguchi method was employed for optimization of key parameters affecting the synthesis of Cu (BTC) . The results indicated that the optimum synthesis conditions with the highest CO selectivity can be obtained using 1 g of ligand, applied voltage of 25 V, synthesis time of 2 h, and electrode length of 3 cm. The single gas sorption capacity of the synthetized microstructure Cu (BTC) for CO (at 298 K and 1 bar) was a considerable value of 4.40 mmol·g . The isosteric heat of adsorption of both gases was calculated by inserting temperature-dependent form of Langmuir isotherm model in the Clausius-Clapeyron equation. The adsorption of CO /N binary mixture with a concentration ratio of 15/85 vol-% was also studied experimentally and the result was in a good agreement with the predicted value of IAST method. Moreover, Cu (BTC) showed no considerable loss in CO adsorption after six sequential cycles. In addition, artificial neural networks (ANNs) were also applied to predict the separation behavior of CO /N mixture by MOFs and the results revealed that ANNs could serve as an appropriate tool to predict the adsorptive selectivity of the binary gas mixture in the absence of experimental data.

关键词: Cu3(BTC)2 electrochemical synthesis     CO2 adsorption     Taguchi optimization     ANN modeling    

The size distribution of airborne bacteria and human pathogenic bacteria in a commercial composting plant

《环境科学与工程前沿(英文)》 2021年 第15卷 第3期 doi: 10.1007/s11783-020-1356-4

摘要:

•Bacterial concentrations from eight stages were 104–105copies/m3.

关键词: Size distribution     Airborne bacteria     Biological diversity     Human pathogenic bacteria     Composting plants    

Construction of nitrogen-doped carbon cladding LiMnO film electrode with enhanced stability for electrochemically

《化学科学与工程前沿(英文)》 2023年 第17卷 第12期   页码 2050-2060 doi: 10.1007/s11705-023-2343-7

摘要: Reducing the dissolution of Mn from LiMn2O4 (LMO) and enhancing the stability of film electrodes are critical and challenging for Li+ ions selective extraction via electrochemically switched ion exchange technology. In this work, we prepared a nitrogen-doped carbon cladding LMO (C-N@LMO) by polymerization of polypyrrole and high-temperature annealing in the N2 gas to achieve the above purpose. The modified C-N@LMO film electrode exhibited lower Mn dissolution and better cyclic stability than the LMO film electrode. The dissolution ratio of Mn from the C-N@LMO film electrode decreased by 42% compared to the LMO film electrode after 10 cycles. The cladding layer not only acted as a protective layer but also functioned as a conductive shell, accelerating the migration rate of Li+ ions. The intercalation equilibrium time of the C-N@LMO film electrode reached within an hour during the extraction of Li+ ions, which was 33% less compared to the pure LMO film electrode. Meanwhile, the C-N@LMO film electrode retained evident selectivity toward Li+ ions, and the separation factor was 118.38 for Li+ toward Mg2+ in simulated brine. Therefore, the C-N@LMO film electrode would be a promising candidate for the recovery of Li+ ions from salt lakes.

关键词: LiMn2O4     lithium extraction     surface coating     cyclic stability     Mn dissolution    

Electroactivity of the magnetotactic bacteria AMB-1 and MSR-1

《环境科学与工程前沿(英文)》 2023年 第18卷 第4期 doi: 10.1007/s11783-024-1808-3

摘要:

● The first study of electrochemically active magnetotactic bacteria.

关键词: Magnetotactic bacteria     Magnetospirillum magneticum     Magnetospirillum gryphiswaldense     Extracellular electron transfer     Microbial fuel cells    

Organic and inorganic phosphorus uptake by bacteria in a plug-flow microcosm

Jinbo ZHAO, Xuehua LIU

《环境科学与工程前沿(英文)》 2013年 第7卷 第2期   页码 173-184 doi: 10.1007/s11783-013-0494-3

摘要: Phosphorus (P) is a vital nutrient for sustaining natural water productivity. Both particulate and dissolved forms of organic and inorganic P are potentially important sources of bioavailable P for primary and secondary producers. A microcosm system to imitate the bacterial community in Plym river sediment and pore water is described and bacterial uptake rates for inorganic and organic phosphorus are presented in this paper. The aim of this study was to investigate the uptake of two organic phosphorus compounds (phytic acid and D-glucose-6-phosphate) by freshwater bacteria. The bioreactors comprise glass columns packed with two types of small glass beads on which bacterial biofilm can develop. The glass beads with different porosity were introduced to simulate River SPM. The selected P compounds spiked into the inflow of the microcosm, and measured the step change of P concentration in the outflow to investigate the behavior of bacterial uptake of nutrients. The results showed that organic phosphorus was converted into inorganic phosphorus but the conversion rate depended on the type of phosphorus species. One experiment suggested that phytic acid (refractory) could displace phosphate from the biofilm surface; the other experiment showed that D-glucose-6-phosphate (labile) could be hydrolysed and utilized easily by the bacteria. The results also suggested that bacteria might break down the C-P bonds to utilize the carbon. Further experiments should investigate the effect of varying the C:N:P ratio in the microcosm system to determine which nutrient limits bacteria uptake.

关键词: organic phosphorus     bacteria     uptake    

Visible light induces bacteria to produce superoxide for manganese oxidation

《环境科学与工程前沿(英文)》 2023年 第17卷 第2期 doi: 10.1007/s11783-023-1619-y

摘要:

● Term of manganese-oxidizing microorganisms should be reconsidered.

关键词: Mn(II) oxidation     Manganese-oxidizing bacteria     Reactive oxygen species     Mn(III/IV) oxides    

Synergistic degradation of pyrene and volatilization of arsenic by cocultures of bacteria and a fungus

Shuang LIU, Yanwei HOU, Guoxin SUN

《环境科学与工程前沿(英文)》 2013年 第7卷 第2期   页码 191-199 doi: 10.1007/s11783-012-0470-3

摘要: The combination of two bacteria ( sp. PY1 and sp. PY2) and a fungus ( sp. PY3), isolated from contaminated soils near a coking plant, were investigated with respect to their capability to degrade pyrene and volatilize arsenic. The results showed that all strains could use pyrene and arsenic as carbon and energy sources in a basal salts medium (BSM), with the combined potential to degrade pyrene and volatilize arsenic. sp. PY1, sp. PY2 and sp. PY3 were isolated from the consortium and were shown to degrade pyrene and volatilize arsenic independently and in combination. Fungal-bacterial coculture has shown that the most effective removal of pyrene was 96.0% and volatilized arsenic was 84.1% after incubation in liquid medium after 9 days culture, while bioremediation ability was 87.2% in contaminated soil with 100 mg·kg pyrene. The highest level of arsenic volatilization amounted to 13.9% of the initial As concentration in contaminated soil after 63 days. Therefore, a synergistic degradation system is the most effective approach to degrade pyrene and remove arsenic in contaminated soil. These findings highlight the role of these strains in the bioremediation of environments contaminated with pyrene and arsenic.

关键词: pyrene     arsenic     bioremediation     bacteria     fungus    

Nitrifying and denitrifying bacteria in aerobic granules formed in sequencing batch airlift reactors

WANG Fang, YANG Fenglin, QI Aijiu

《环境科学与工程前沿(英文)》 2007年 第1卷 第2期   页码 184-189 doi: 10.1007/s11783-007-0032-2

摘要: The purpose of this study was to investigate nitrifying bacteria and denitrifying bacteria isolated from aerobic granules. Aerobic granules were formed in an internal-circulate sequencing batch airlift reactor (SBAR) and biodegradation of NH3--N was analyzed in the reactor. Bacteria were isolated and determined from aerobic granules using selected media. The growth properties and morphology of bacteria colonies were observed by controlling aerobic or anaerobic conditions in the culture medium. It was found that bacteria in aerobic granules were diverse and some of them were facultative aerobes. The diversity of bacteria in aerobic granules was a premise of simultaneous nitrification and denitrification.

Airborne bacteria associated with particulate matter from a highly urbanised metropolis: A potential

《环境科学与工程前沿(英文)》 2022年 第16卷 第9期 doi: 10.1007/s11783-022-1552-5

摘要:

• The airborne bacteria of Mexico City are representative of urban environments.

关键词: Airborne bacteria     Urbanisation     PM10     Mexico City     Microbiome    

Synergistic effects of sodium hypochlorite disinfection and iron-oxidizing bacteria on early corrosion

《环境科学与工程前沿(英文)》 2022年 第16卷 第6期 doi: 10.1007/s11783-021-1506-3

摘要:

• The early corrosion process in the cast iron pipes was investigated.

关键词: Cast iron pipe corrosion     Drinking water distribution systems     Chlorine disinfection     Iron-oxidizing bacteria     Coupling effects    

Magnetotactic bacteria: Characteristics and environmental applications

Xinjie Wang, Yang Li, Jian Zhao, Hong Yao, Siqi Chu, Zimu Song, Zongxian He, Wen Zhang

《环境科学与工程前沿(英文)》 2020年 第14卷 第4期 doi: 10.1007/s11783-020-1235-z

摘要: • Magnetotactic bacteria (MTB) synthesize magnetic nanoparticle within magnetosomes. • The morphologic and phylogenetic diversity of MTB were summarized. • Isolation and mass cultivation of MTB deserve extensive research for applications. • MTB can remove heavy metals, radionuclides, and organic pollutants from wastewater. Magnetotactic bacteria (MTB) are a group of Gram-negative prokaryotes that respond to the geomagnetic field. This unique property is attributed to the intracellular magnetosomes, which contains membrane-bound nanocrystals of magnetic iron minerals. This review summarizes the most recent advances in MTB, magnetosomes, and their potential applications especially the environmental pollutant control or remediation. The morphologic and phylogenetic diversity of MTB were first introduced, followed by a critical review of isolation and cultivation methods. Past research has devoted to optimize the factors, such as oxygen, carbon source, nitrogen source, nutrient broth, iron source, and mineral elements for the growth of MTB. Besides the applications of MTB in modern biological and medical fields, little attention was made on the environmental applications of MTB for wastewater treatment, which has been summarized in this review. For example, applications of MTB as adsorbents have resulted in a novel magnetic separation technology for removal of heavy metals or organic pollutants in wastewater. In addition, we summarized the current advance on pathogen removal and detection of endocrine disruptor which can inspire new insights toward sustainable engineering and practices. Finally, the new perspectives and possible directions for future studies are recommended, such as isolation of MTB, genetic modification of MTB for mass production and new environmental applications. The ultimate objective of this review is to promote the applications of MTB and magnetosomes in the environmental fields.

关键词: Magnetotactic bacteria     Magnetosome     Heavy metal     Radionuclide     Organic pollutants    

advanced engineering measures on displacement and stress field of surrounding rock in tunnels crossing active

《结构与土木工程前沿(英文)》 doi: 10.1007/s11709-023-0966-x

摘要: Based on significant improvements in engineering materials, three advanced engineering measures have been proposed—super anchor cables, high-strength concrete anti-fault caverns, and grouting modification using high-strength concrete-to resist fault dislocation in the surrounding rock near tunnels crossing active strike-slip faults. Moreover, single- or multiple-joint advanced engineering measures form the local rock mass-anti-fault (LRAF) method. A numerical method was used to investigate the influence of LRAF methods on the stress and displacement fields of the surrounding rock, and the anti-fault effect was evaluated. Finally, the mechanism of action of the anchor cable was verified using a three-dimensional numerical model. The numerical results indicated that the anchor cable and grouting modification reduced the displacement gradient of the local surrounding rock near the tunnels crossing fault. Furthermore, anchor cable and grouting modifications changed the stress field of the rock mass in the modified area. The tensile stress field of the rock mass in the modified anchor cable area was converted into a compressive stress field. The stress field in the modified grouting area changed from shear stress in the fault slip direction to tensile stress in the axial tunnel direction. The anti-fault cavern resisted the dislocation displacement and reduced the maximum dislocation magnitude, displacement gradient, and shear stress. Among the three advanced engineering measures, the anchor cable was the core of the three advanced engineering measures. An anchor cable, combined with other LRAF measures, can form an artificial safety island at the cross-fault position of the rock mass to protect the tunnel. The research results provide a new supporting idea for the surrounding rock of tunnels crossing active strike-slip faults.

关键词: anti-fault effect     engineering measures     LRAF method     stress and displacement field     tunnel-crossing active faults    

Effect of denitrifying bacteria on the electrochemical reaction of activated carbon fiber in electrochemical

YING Diwen, JIA Jinping, ZHANG Lehua

《环境科学与工程前沿(英文)》 2007年 第1卷 第3期   页码 305-310 doi: 10.1007/s11783-007-0051-z

摘要: An electrochemical-activated denitrifying biofilm system consisting of activated carbon fiber electrodes immobilized with denitrifying bacteria film as cathode was studied. A revised model for an electrochemical-activated denitrifying biofilm was developed and validated by electrochemical analysis of cathodal polarization curves and nitrate consumption rate. The cathodal polarization curve and nitrate consumption rate were introduced to verify the rate of electrochemical reaction and the activity of denitrifying bacteria, respectively. It was shown that the denitrification process effectively strengthened the electrochemical reaction while the electron also intensified denitrification activity. Electron was transferred between electrochemical process and biological process not only by hydrogen molecule but also by new produced active hydrogen atom. Additionally, a parameter of apparent exchange current density was deprived from the cathodal polarization curve with high overpotential, and a new bio-effect current density was defined through statistical analysis, which was linearly dependent to the activity of denitrification bacteria. Activated carbon fiber (ACF) electrode was also found to be more suitable to the electrochemical denitrifying system compared with graphite and platinum.

关键词: ACF     apparent exchange     hydrogen molecule     activated     biological process    

标题 作者 时间 类型 操作

Response of indigenous Cd-tolerant electrochemically active bacteria in MECs toward exotic Cr(VI) based

Xia Hou, Liping Huang, Peng Zhou, Hua Xue, Ning Li

期刊论文

An antibiotic composite electrode for improving the sensitivity of electrochemically active biofilm biosensor

期刊论文

Optimization of electrochemically synthesized Cu

Kasra Pirzadeh, Ali Asghar Ghoreyshi, Mostafa Rahimnejad, Maedeh Mohammadi

期刊论文

The size distribution of airborne bacteria and human pathogenic bacteria in a commercial composting plant

期刊论文

Construction of nitrogen-doped carbon cladding LiMnO film electrode with enhanced stability for electrochemically

期刊论文

Electroactivity of the magnetotactic bacteria AMB-1 and MSR-1

期刊论文

Organic and inorganic phosphorus uptake by bacteria in a plug-flow microcosm

Jinbo ZHAO, Xuehua LIU

期刊论文

Visible light induces bacteria to produce superoxide for manganese oxidation

期刊论文

Synergistic degradation of pyrene and volatilization of arsenic by cocultures of bacteria and a fungus

Shuang LIU, Yanwei HOU, Guoxin SUN

期刊论文

Nitrifying and denitrifying bacteria in aerobic granules formed in sequencing batch airlift reactors

WANG Fang, YANG Fenglin, QI Aijiu

期刊论文

Airborne bacteria associated with particulate matter from a highly urbanised metropolis: A potential

期刊论文

Synergistic effects of sodium hypochlorite disinfection and iron-oxidizing bacteria on early corrosion

期刊论文

Magnetotactic bacteria: Characteristics and environmental applications

Xinjie Wang, Yang Li, Jian Zhao, Hong Yao, Siqi Chu, Zimu Song, Zongxian He, Wen Zhang

期刊论文

advanced engineering measures on displacement and stress field of surrounding rock in tunnels crossing active

期刊论文

Effect of denitrifying bacteria on the electrochemical reaction of activated carbon fiber in electrochemical

YING Diwen, JIA Jinping, ZHANG Lehua

期刊论文